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I've tried setting org.gnome.desktop.input-sources to ['space:ctrl'] but it doesn't work.

Note: I want the spacebar to keep working as before (Space should trigger both Ctrl and Space, I don't mind the conflict).

1 Answers1

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From a terminal run:

xmodmap -e 'keycode 65=Control_R'

To undo, type:

xmodmap -e 'keycode 65=space'

In general, to see the list of all keysyms that you can map and their names, type:

xmodmap -pk