For angles, radians are the natural unit, because:
$$ \frac d {d\theta} \cos\theta = -\sin\theta $$
while
$$ \frac d {d\theta}\cos(\frac{\pi}{180^{\circ}}\theta) = -\frac{\pi}{180^{\circ}}\sin(\frac{\pi}{180^{\circ}}\theta)$$
which gets messy fast.
Moreover, there are $2\pi$ radians, and the circumference of the unit circle is $2\pi$.
Likewise for solid angle, the surface area the unit sphere is $4\pi$, which is also the total solid angle.
One can use square degrees, the moon subtends something like $\pi/16$ degrees squared, but that only work out well because it is so small. The whole sky is something like 40,000 degrees-squared, but feel free to calculate the exact value. The exercise should dissuade you from worrying about square degrees.
On geodetic coordinates: I've heard navigators, who did not have electronic computation, liked 360 because its numerous divisors. Note that latitude and longitude are not angles. They can be associated with angles, and the various latitudes (geodetic, parametric, authalic, rectifying, geocentric) are all different...but they are coordinates, and should never be expressed in radians.