No you can't reconstruct the shape just from the mass moment of inertia (MMOI) values. At most you can get 3 eigenvalues (the principal moments of inertia) and an orientation matrix which diagonalizes the MMOI matrix.
Finding the MMOI values from a shape involves a triple integral over the volume and integration (like any other summation process) loses information. It is a sort of averaging process. If you know the average weight of two people you can't deduce anything about the individual weights without additional information for example. That is because the averaging process loses information.
From the diagonalized MMOI matrix with principal values $I_1$, $I_2$ and $I_3$ in decreasing order you can find an equivalent solid ellipsoid with the following semi-major radiuses
$$\begin{aligned}
r_1 & = \sqrt{ \frac{5}{2 m} | I_2 + I_3 - I_1 | } \\
r_2 & = \sqrt{ \frac{5}{2 m} | I_1 - I_2 - I_3 | } \\
r_3 & = \sqrt{ \frac{5}{2 m} | I_1 + I_2 - I_3 | }
\end{aligned}$$